Impact of distinct sintering temperatures in pellets to strontium immobilization

Authors

DOI:

https://doi.org/10.15392/2319-0612.2024.2652

Keywords:

niobium , zeolite , liquido effluent, strontium immobilization

Abstract

The immobilization of radioactive strontium (Sr) from liquid effluents, a byproduct of nuclear fission and accidents, presents significant environmental and public health challenges. This study evaluates the immobilization of Sr in a glass matrix by comparing the effects of different sintering temperatures. The analyses started from three temperatures 800ºC, 900ºC and 1000ºC for each of the four compositions, which vary the addition of niobium (Nb) content in the vitreous matrix by 2%, 4%, 6% and 8% in mol. The highest temperature was excluded because its deformation did not match the final objective, at 900ºC the compositions had better results in density and water absorption, so that at the same temperature the composition with 4% niobium responded better to the results. The study underscores the significance of treating temperature and Nb content in the glass matrix for effective Sr immobilization, offering valuable insights for the development of safe and sustainable nuclear waste management strategies.

Downloads

Download data is not yet available.

References

[1] World Nuclear Waste Report. The World Nuclear Waste Report - Focus Europe. Disponível em: https://worldnuclearwastereport.org/. Acesso em: 29 out. 2024.

[2] INAN, S. Inorganic ion exchangers for strontium removal from radioactive waste: a review. J Radioanal Nucl Chem, v. 331, n. 03, p. 1137-1154, 2022. DOI: https://doi.org/10.1007/s10967-022-08206-3

[3] BURGER, A.; LICHTSCHEIDL, I. Strontium in the environment: Review about reactions of plants towards stable and radioactive strontium isotopes. Science of The Total Environment, Vienna, v. 653, p. 1458-1512, 2019. DOI: https://doi.org/10.1016/j.scitotenv.2018.10.312

[4] LI, L.; et al. Immobilization of strontium and cesium by aluminosilicate ceramics derived from metakaolin geopolymer-zeolite A composites via 1100 °C heating treatment. Ceram Int, v. 48, n. 11, p. 15236–15242, 2022. DOI: https://doi.org/10.1016/j.ceramint.2022.02.054

[5] COSTA-SILVA, D. L.; BARTOLOMÉ, J. F.; SILVA, A. C.; MELLO-CASTANHO, S. Structural and thermal influence of niobia in aluminoborosilicate glasses. Ceram Int, v. 48, n. 13, p. 18433–18440, 2022. DOI: https://doi.org/10.1016/j.ceramint.2022.03.112

[6] IZIDORO, J. C.; CASTANHO, D. ; et al. Application of high-purity zeolite A synthesized from different coal combustion by-products in carbon dioxide capture. Int J Environ Impacts, v. 02, n. 03, p. 215-228, 2019. DOI: https://doi.org/10.2495/EI-V2-N3-215-228

[7] COSTA-SILVA, D. L.; ARAUJO, M. S.; FUNGARO, D. A.; SILVA, P. S. C.; MELLO-CASTANHO, S. New approach to niobia-modified borosilicate glasses for Cs waste immobilization. J Materials Research and Technology, v. 31, p. 1229-1235, 2024. DOI: https://doi.org/10.1016/j.jmrt.2024.06.099

[8] ASTM – American Society for Testing and Materials. Standard Test Method for Water Absorption, Bulk Density, Apparent Porosity, and Apparent Specific Gravity of Fired Whiteware Products, ASTM - C373-88. 2006.

Downloads

Published

2025-02-17

How to Cite

Impact of distinct sintering temperatures in pellets to strontium immobilization. Brazilian Journal of Radiation Sciences, Rio de Janeiro, Brazil, v. 12, n. 4A (Suppl.), p. e2652, 2025. DOI: 10.15392/2319-0612.2024.2652. Disponível em: https://bjrs.org.br/revista/index.php/REVISTA/article/view/2652. Acesso em: 22 feb. 2025.

Similar Articles

21-27 of 27

You may also start an advanced similarity search for this article.

Most read articles by the same author(s)