Preliminary measurements using a Triple to Double Coincidence Ratio (TDCR) Liquid Scintillator Counter System
DOI:
https://doi.org/10.15392/bjrs.v9i1A.1512Keywords:
Carbon-14, Liquid scintillation, Tracer technique, TDCR.Abstract
The preliminary measurements using a Triple to Double Coincidence Ratio (TDCR) Liquid Scintillator Counter System developed by the Nuclear Metrology Laboratory (LMN) at IPEN, is presented. The TDCR system makes use of three photomultipliers positioned at 120° relative angle, operating in coincidence. For this preliminarymeasurement, 14C was selected to be standardized; 14C was chosen due to be a pure beta emitter with low end-point energy of 156 keV, which is suitable to be measured by the TDCR system. This solution was previously calibrated by the efficiency tracing technique using a 4p(PC)b-g coincidence system, employing 60Co as a tracer. The activity of the 14C solution by efficiency tracing technique was determined by using the extrapolation technique, changing the beta efficiency by pulse height discrimination. In order to determine the final activity, a Monte Carlo simulation was used to generate the extrapolation curve. The Software Coincidence System (SCS) developed by the LMN was used for both systems to register the events. MICELLE 2 code was used to calculate the theoretical TDCR efficiency. Measurements using HIDEX, a commercial liquid scintillator system, were also carried out and the results from the three methods were compared, showing a good agreement.
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References
BE, M.-M.; et al., C-14 Accessed at http://www.nucleide.org/DDEP_WG/DDEPdata.htm. 2015.
KOSKINAS, M. F.; PIRES, C. A.; YAMAZAKI, I. M.; SILVA, E. A.; DIAS, M. S.; Standardization of 55Fe by tracing method. Appl. Radiat. Isot, 66, p.733-736, 2008.
BAERG, A. P. The efficiency extrapolation method in coincidence counting. Nucl. Instrum. Methods 112, p 143–150, 1973.
TOLEDO, F.; BRANCACCIO, F.; LAPOLLI, A.; DIAS. M. S. Design of Electronic System with Simultaneous Registering of Pulse and Event Time Applied to 4pib-g Coincidence Method. Proceedings of the IEEE 2008 Nuclear Science Symposium, Medical Imaging Conference and 16th Room Temperature Semiconductor Detector Workshop Dresden, Germany 19 - 25 October in CDROM, 2008.
DIAS, M. S., KOSKINAS, M. F. Standardization of a Tl-204 radioactive solution. Appl. Radiat. and Isot., 58, p. 235-238, 2003.
DIAS, M.S.; TAKEDA, M. N.; KOSKINAS, M.F. Application of Monte Carlo simulation to the prediction of extrapolation curves in the coincidence technique. Appl. Radiat. Isot, 64, p.1186-1192, 2006.
ORNL, Monte Carlo N-Particle Transport Code System, MCNP5, RSICC Computer Code Collection, Oak Ridge National Laboratory. 2006.
Annunziata, M. L. Handbook of Radioactivity Analysis. 3a Ed., Academic Press, 2012.
BRODA, R. A.; CASSETTE, P.; KOSSERT, K. Radionuclide metrology using liquid scintillation counting. Metrologia, 44, S36-S52, 2007.
BRODA, R. A. A review of the triple-to-double coincidence ratio (TDCR) method for standardization radionuclides. Appl. Radiat. Isot. 58, p.585-594, 2003.
KOSSERT, K.; GRAU CHARLES, A. Improved method for the calculation of the counting efficiency of electron-capture nuclides in liquid scintillation samples. Appl.Radiat.Isot. 68, p. 1482-1488, 2010.
National Instruments, 2013. http://www.ni.com/manuals/ (accessed March 2013.
DIAS, M. S. SCTAC, Version 6.0 – User´s Manual. Internal Report, Nuclear Metrology La-boratory, IPEN-CNEN/SP, 2014.
MOREIRA, D. S. LSCALC01G – User´s Manual. Internal Report, Nuclear Metrology Laboratory, IPEN-CNEN/SP, 2019.
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