Assessment of Sr-90 in water samples: precision and accuracy

Authors

  • Marcelo Bessa Nisti Instituto de Pesquisas Energéticas e Nucleares IPEN-CNEN/SP
  • Cátia H.R. Saueia IPEN-CNEN/SP
  • Bruna Castilho IPEN-CNEN/SP
  • Barbara P. Mazzilli IPEN-CNEN/SP

DOI:

https://doi.org/10.15392/bjrs.v7i2A.559

Keywords:

Sr-90, LSC, precision, accuracy

Abstract

The study of artificial radionuclides dispersion into the environment is very important to control the nuclear waste discharges, nuclear accidents and nuclear weapons testing. The accidents in Fukushima Daiichi Nuclear Power Plant and Chernobyl Nuclear Power Plant, released several radionuclides in the environment by aerial deposition and liquid discharge, with various level of radioactivity. The 90Sr was one of the elements released into the environment. The 90Sr is produced by nuclear fission with a physical half-life of 28.79 years with decay    energy of 0.546 MeV. The aims of this study are to evaluate the precision and accuracy of three methodologies for the determination of 90Sr in water samples: Cerenkov, LSC direct method and with radiochemical            separation. The performance of the methodologies was evaluated by using two scintillation counters (Quantulus and Hidex). The parameters Minimum Detectable Activity (MDA) and Figure Of Merit (FOM) were determined for each method, the precision and accuracy were checked using 90Sr standard solutions. 

Downloads

Download data is not yet available.

References

L´ANNUNZIATA, M. F. Handbook of Radioactivity Analysis, 3rd ed. Academic Press: Elsevier, 2012.

IAEA - International Atomic Energy Agency. The Fukushima Daiichi accident - Technical volume 4 - Radiological consequences, ed. Vienna: International Atomic Energy Agency, 2015.

PACKARD. Handbook of Environmental Liquid Scintillation Spectrometry – A Compilation of Theory and Methods, ed. Packard – A Canberra Company, USA, 1994.

QUANTULUS. Instrument Manual-Wallac 1220 QuantulusTM Ultra Low Level Liquid Scintillation Spectrometer, ed. PerkinElmer, 2009.

HIDEX. Handbook 425-201 Automatic Liquid Scintillation Counter, Hidex 300SL, ed. Hidex, 2008.

PERKINELMER. Liquid Scintillation Analysis - Science and Technology, <http://www.perkinelmer.co.jp/Portals/0/resource/products_ls/ls_cocktails/pdf/LSABooklet_012129_01.pdf, 2015.

CHYLIŃSKI, A.; BRODA, R.; RADOSZEWSKI, T. The National Standard Unit of Radionuclide Activity and the related standards in Poland, NUKLEONIKA, v. 48(1), p. 51-55, 2003.

CASSETTE, P.; GRIGORESCU, E. L.; RAZDOLESCU, A. C. Obtaining tritiated water standards using triple to double coincidence ratio (tdcr) method, Report WP7 IDRANAP 26-02, p. 2-7, 2002.

OLFERT, J, M.; DAI X.; KRAMER-TREMBLAY, S. Rapid determination of 90Sr/90Y in water samples by liquid scintillation and Cherenkov counting, Journal of Radioanalytical and Nuclear Chemistry, v.300, p.263-267, 2014.

CURRIE, L.A. Limits for qualitative detection and quantitative determination”. Analytical Chemistry, v. 40, p.586-593, 1968.

VIANNA, M.E.; TAUHATA, L.; OLIVEIRA, J.P.; OLIVEIRA, A.E.; GARCIA, L. C.; CONCEIÇÃO, C.S.; CLAIN, A. F. Quality of radionuclide analysis in environ-mental samples. Applied Radiation and Isotopes, v.173/174, p.15-18, 1995.

TAUHATA, L.; VIANNA, M.E.C.M.; OLIVEIRA, A.E.; FERREIRA, A.C.M.; BRAGANÇA, M.J.C.S.; CLAIN, A. F. The influence of uncertainties of measure-ments in laboratory performance evaluation using an intercomparison program of radio-nuclide assays in environmental samples. Applied Radiation and Isotopes, v. 64, p.1174-1178, 2006.

Downloads

Published

2019-02-06

Issue

Section

The Meeting on Nuclear Applications (ENAN)

How to Cite

Assessment of Sr-90 in water samples: precision and accuracy. Brazilian Journal of Radiation Sciences, Rio de Janeiro, Brazil, v. 7, n. 2A (Suppl.), 2019. DOI: 10.15392/bjrs.v7i2A.559. Disponível em: https://bjrs.org.br/revista/index.php/REVISTA/article/view/559.. Acesso em: 21 nov. 2024.

Similar Articles

1-10 of 126

You may also start an advanced similarity search for this article.

Most read articles by the same author(s)