Re-characterization of pneumatic station position for short irradiations of IEA-R1 reactor for use in k0-method

Authors

DOI:

https://doi.org/10.15392/2319-0612.2026.2701

Keywords:

k0-INAA, neutron activation method, neutron flux

Abstract

This work presents the re-characterization of pneumatic station irradiation position of IEA-R1 reactor for use in k0-INAA method. The thermal-epithermal neutron flux ratio f and the epithermal neutron flux distribution factor α of the IPEN IEA-R1 reactor were determined at the pneumatic irradiation station. To obtain these values, the “bare triple monitor” method was used with 198Au –97Zr – 95Zr.  To evaluate its reproducibility, the temporal variation of these parameters was analyzed, with validation carried out through irradiation of reference materials of geological origin G-S-N (granite) and biological INCT-MPH-2 (mix of herbs). The results obtained for f  and α show that such values ​​are reproducible and compatible with each other, according to the normal Gaussian distribution for up to 1 standard deviation of confidence. The results obtained for the elements detected in the samples agree with the recommended values, with relative errors (bias) less than 10%, except in the case of Mn in G-S-N (16.3%). These results indicate that it is possible to routinely use this method for LAN-IPEN researchers to analyze geological and biological samples.

Downloads

Download data is not yet available.

Author Biography

  • João Pedro Oliveira Flores, Nuclear Energy Research Institute
    Física Nuclear/Tecnologia Nuclear

References

SIMONITS, A.; DE CORTE, F.; HOSTE, J.; Single-Comparator methods in reactor neutron activation analysis. Journal of Radioanalytical and Nuclear Chemistry, v. 24, p. 31-46, 1975. DOI: https://doi.org/10.1007/BF02514380

LANGE, C. N.; CAMARGO, I. M. C.; FIGUEIREDO, A. M. G. M.; CASTRO, L.; VASCONCELLOS, M. B. A.; TICIANELLI, R. B. A Brazilian coal fly ash as a potential source of rare earth elements. Journal of Radioanalytical and Nuclear Chemistry, v. 311, p. 1235-1241, 2017. DOI: https://doi.org/10.1007/s10967-016-5026-8

DE CORTE, F. The k0-Standardization Method: A move to the optimisation of neutron activation analysis, Rijksuniversiteit Gent, Faculteit Van de Wetenschappen, Gent, Belgium, 1986.

DE CORTE, F.; MOENS, L.; SIMONITS, A.; DE WISPERLAERE, A.; HOSTE, J. Instantaneous

FLORES, J. P. O.; SILVA, P. S. C.; DIAS, M. S.; KOSKINAS, M. F.; MOREIRA, D. S.; YAMAZAKI, I. M. Calibration of the short irradiation facility for k0 - NAA implementation at the IEA-R1 reactor. Brazilian Journal of Radiation Sciences, 9(1A), São Paulo, 2021. DOI: https://doi.org/10.15392/bjrs.v9i1A.1570

DE CORTE, F.; SIMONITS, A. Recommended nuclear data for use in the k0 standardization of neutron activation analysis. At. Data Nucl. Data Tables, v. 85, p. 47-67, 2003. DOI: https://doi.org/10.1016/S0092-640X(03)00036-6

PUERTA, C. D. Aplicação do método k0-INAA no laboratório de análise por ativação com nêutrons do Ipen utilizando o programa k0-IAEA. Análise de amostras biológicas. 2013. 202 f. Dissertação (Mestrado em Tecnologia Nuclear), Instituto de Pesquisas Energéticas e Nucleares, IPEN-CNEN, São Paulo. Disponível em: ‹http://repositorio.ipen.br/› (data de consulta no formato: 16/02/2024).

Jaćimović R, k0 Database, available in: https://www.kayzero.com/k0naa/k0naaorg/Nuclear_Data_SC/Entries/2020/8/24_Update_of_k0-database_I-128.html. Accessed: 05 May 2022.

IAEA – International Atomic Energy Agency. Proficiency Testing by Interlaboratory Comparison: Analytical Laboratories in Nuclear Institutions. IAEA-TECDOC-1210, Vienna, 2001.

BLAND, J.; ALTMAN M. D. G. Statistical methods for assessing agreement between two methods of clinical measurement. The Lancet, v. 327, n. 8476, p. 307–310, 1986. DOI: https://doi.org/10.1016/S0140-6736(86)90837-8

Downloads

Published

2026-02-27

Issue

Section

Original Articles

Categories